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    桂中坳陷早石炭世泥页岩地球化学特征及近源气成藏模式

    王保忠 欧文佳 王传尚 彭中勤 张国涛

    王保忠, 欧文佳, 王传尚, 彭中勤, 张国涛, 2018. 桂中坳陷早石炭世泥页岩地球化学特征及近源气成藏模式. 地球科学, 43(7): 2222-2233. doi: 10.3799/dqkx.2018.226
    引用本文: 王保忠, 欧文佳, 王传尚, 彭中勤, 张国涛, 2018. 桂中坳陷早石炭世泥页岩地球化学特征及近源气成藏模式. 地球科学, 43(7): 2222-2233. doi: 10.3799/dqkx.2018.226
    Wang Baozhong, Ou Wenjia, Wang Chuanshang, Peng Zhongqin, Zhang Guotao, 2018. Geochemical Characteristics of the Early Carboniferous Shale in Guizhong Depression and Their Contribution to Adjacent Gas Reservoirs. Earth Science, 43(7): 2222-2233. doi: 10.3799/dqkx.2018.226
    Citation: Wang Baozhong, Ou Wenjia, Wang Chuanshang, Peng Zhongqin, Zhang Guotao, 2018. Geochemical Characteristics of the Early Carboniferous Shale in Guizhong Depression and Their Contribution to Adjacent Gas Reservoirs. Earth Science, 43(7): 2222-2233. doi: 10.3799/dqkx.2018.226

    桂中坳陷早石炭世泥页岩地球化学特征及近源气成藏模式

    doi: 10.3799/dqkx.2018.226
    基金项目: 

    中国地质调查局项目 DD20160179

    详细信息
      作者简介:

      王保忠(1980-), 男, 工程师, 博士, 从非常规油气综合研究及区域地质调查工作, 主要从事页岩在高演化阶段的生烃富集机理研究

      通讯作者:

      欧文佳

    • 中图分类号: P595;P597

    Geochemical Characteristics of the Early Carboniferous Shale in Guizhong Depression and Their Contribution to Adjacent Gas Reservoirs

    • 摘要: 目前针对桂中坳陷早石炭世富有机质泥页岩的生烃潜力方面研究很少,严重制约了该区以页岩气为主的非常规油气勘探.本研究对鹿寨县城西石炭系鹿寨组泥页岩系统取样分析,从有机碳含量、岩石热解、有机碳同位素组成、抽提物正构烷烃组成特征及泥岩镜质体反射率多个方面讨论了该套泥页岩的生烃潜力;结合区域构造演化史总结了与下石炭统岩关阶泥页岩密切相关的3种近源气藏赋存模式.研究结果表明:泥页岩的TOC值分布于0.25%~15.67%,其中强制海退前沉积的泥页岩富含有机质,TOC值均大于2%,TOC值与氯仿沥青"A"、生烃潜量及总烃呈弱正相关关系.泥页岩的有机质类型主体为Ⅱ型;泥页岩的Ro值分布于1.72%~2.78%,处于过成熟阶段.泥页岩上下岩性组合特征及桂中坳陷现今所处的构造位置表明,坳陷中部对冲构造区为有利的近源气藏形成区,背冲构造区为较差区;坳陷边缘逆冲推覆构造区为存在岩性圈闭的近源气藏形成区.

       

    • 图  1  桂中坳陷早石炭世沉积相简图

      焦大庆等(2003)梅冥相等(2004)修改

      Fig.  1.  Sedimentary facies diagram of Guizhong depression Early Carboniferous

      图  2  研究区早石炭世三级层序岩性特征

      a.SQ2含硅质泥岩断口特征;b.SQ3底部滑塌构造及新鲜泥岩样品特征;c.SQ01/2层界线及2层瘤状灰岩特征;d.SQ1碳质页岩风化特征及新鲜样品沿页理剥落

      Fig.  2.  Lithologic characteristics of Early Carboniferous the 3rd grade sequence in the study area

      图  3  鹿寨县下石炭统鹿寨组取样剖面分层及层序划分

      Fig.  3.  Stratification and sequence division of sampling profile in the Lower Carboniferous Luzhai Formation, in Luzhai County

      图  4  样品C1lz-5-1饱和烃TIC、m/z=217及m/z=191质量色谱图

      Fig.  4.  TIC, m/z=217 and m/z=191 mass chromatograms of saturated hydrocarbon from sample C1lz-5-1

      图  5  鹿寨组不同层段泥页岩Pr/nC17和Ph/nC18关系

      Yandoka et al.(2015)

      Fig.  5.  Relationship between Pr/nC17 and Ph/nC18 of carbonaceous shale in different strata in Luzhai Formation

      图  6  桂中坳陷早石炭世泥页岩有机碳同位素组成与有机碳含量关系

      Fig.  6.  Relationship between organic carbon isotopic composition and organic carbon content of shale in Early Carboniferous in Guizhong depression

      图  7  桂中坳陷早石炭世泥页岩在不同时期不同构造区域的油气藏形成模式

      Fig.  7.  Formation model of oil and gas reservoir of Early Carboniferous carbonaceous shales in Guizhong depression at different periods and tectonic regions

      表  1  鹿寨长胜凹剖面泥页岩有机质丰度分布特征

      Table  1.   Organic matter abundance distribution of shale in Changshengwa profile in Luzhai County

      样号编号TOC(%)HI(10-3)“A”(%)HC(10-6)S1+S2(10-3)HC/TOC
      C1lz-24-10.476.40.02411.090.0323.6
      C1lz-23-10.313.20.00731.160.03100.5
      C1lz-22-10.577.00.00626.380.0646.3
      C1lz-21-10.513.90.00715.250.0329.9
      C1lz-20-10.946.40.00317.710.0818.8
      C1lz-19-10.434.70.0023.720.038.7
      C1lz-18-20.254.00.0026.320.0125.3
      C1lz-17-11.146.10.0056.260.135.5
      C1lz-16-10.797.60.0036.770.098.6
      C1lz-14-11.061.90.1105.850.035.5
      C1lz-13-12.523.20.00410.210.164.1
      C1lz-10-22.012.00.1765.820.042.9
      C1lz-10-13.801.30.00214.970.063.9
      C1lz-8-24.532.00.1645.540.111.2
      C1lz-7-34.503.10.01522.020.314.9
      C1lz-7-13.053.00.1329.380.153.1
      C1lz-6-34.572.00.1538.820.131.9
      C1lz-5-14.101.50.1406.900.121.7
      C1lz-4-115.676.80.01621.061.251.3
      C1lz-3-1//0.0015.69//
      注:HI(氢指数)=热解烃/有机碳含量;HC(总烃)=饱和烃含量+芳烃含量.
      下载: 导出CSV

      表  2  早石炭世泥页岩链烷烃系列及部分甾烷特征

      Table  2.   The parameters of chain alkane and steranes in the Early Carboniferous shale

      样号编号C21-/C22+Pr/PhPr/nC17Ph/nC18C27R/C29RC28R/C29R
      C1lz-24-111.220.710.470.851.330.92
      C1lz-23-126.610.971.191.911.510.66
      C1lz-22-129.990.780.691.331.110.70
      C1lz-21-121.450.840.511.441.300.65
      C1lz-20-10.960.301.151.401.270.74
      C1lz-19-11.901.28151.903.041.710.58
      C1lz-18-23.771.011.371.031.520.62
      C1lz-17-11.710.94250.85239.321.130.51
      C1lz-16-13.861.03143.812.041.310.60
      C1lz-14-13.571.401.071.091.140.23
      C1lz-13-15.010.870.861.131.380.62
      C1lz-10-21.690.830.871.591.670.86
      C1lz-10-12.430.751.001.241.380.82
      C1lz-8-21.340.921.191.071.190.84
      C1lz-7-3/1.142.492.39//
      C1lz-7-11.781.603.681.630.880.19
      C1lz-6-36.720.830.962.181.250.81
      C1lz-5-11.170.671.331.811.360.80
      C1lz-4-12.930.670.541.211.800.72
      C1lz-3-11.290.912.141.191.920.65
      C1lz-ND-31.801.202.451.161.460.69
      C1lz-ND-22.481.110.800.901.880.94
      C1lz-ND-13.541.220.961.06//
      下载: 导出CSV

      表  3  早石炭世泥页岩显微组成鉴定结果

      Table  3.   Microscopic identification of the shales in the Early Carboniferous

      样号编号腐泥组壳质组镜质组惰质组TI有机质类型
      C1lz-5-19008282.00
      C1lz-7-180015269.751
      C1lz-10-270024646.001
      C1lz-17-1018811-76.50
      C1lz-24-1308512-72.75
      下载: 导出CSV

      表  4  桂中坳陷上古生界泥页岩样品镜质体反射率

      Table  4.   Vitrinite reflectance of shale in the Upper Paleozoic in Guizhong Depression

      采样地点岩性样品数(块)层位Ro(%)
      长胜凹剖面泥岩、页岩5C11.7~2.8
      *上林泥岩9C11.9~2.5
      *鹿寨泥岩、页岩12C11.6~1.9
      *桂林泥岩、页岩4C12.0~3.0
      *象州页岩10D21.0~3.0
      *南丹、河池泥岩3C12.0~3.0
      注:标“*”号样品据黄羚等(2012).
      下载: 导出CSV

      表  5  桂中坳陷泥盆系-下石炭统泥页岩粘土矿物含量及组成特征

      Table  5.   Clay content and composition of shale in the Devonian-Lower Carboniferous in Guizhong Depression

      采样地点岩性样品数
      (块)
      层位粘土矿物含量
      (%)
      主要粘土矿物相对含量
      II/SS
      1石门、环江泥岩、页岩3C1/60~6413~315~27
      2上林泥岩9C11~3 74~8910~205
      2鹿寨泥岩、页岩12C140~70 10~3040~6010~15
      2桂林泥岩、页岩4C131~39 23~3460~7415
      2南丹、河池泥岩3D125~40 >75//
      注:1潘仁芳等(2014)2黄羚等(2012).
      下载: 导出CSV
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