大别山皇城山银矿区及外围陈棚组火山岩U-Pb年代学、地球化学和成矿构造背景

朱江; 吴昌雄; 彭三国; 彭练红; 张闯; 刘锦明

doi:10.3799/dqkx.2018.187

大别山皇城山银矿区及外围陈棚组火山岩U-Pb年代学、地球化学和成矿构造背景

doi: 10.3799/dqkx.2018.187

朱江^1,2,,
吴昌雄³,
彭三国^1,2,
彭练红^1,2,
张闯³,
刘锦明³

1.
中国地质调查局武汉地质调查中心, 湖北武汉 430205
2.
中国地质调查局花岗岩成岩成矿地质研究中心, 湖北武汉 430205
3.
湖北省地质局第六地质大队, 湖北孝感 432000

基金项目:

中国地质调查局项目 121201009000150013

中国地质调查局项目 121201009000160902

详细信息

作者简介:
朱江(1985-), 男, 博士, 高级工程师, 主要从事矿床学、矿产普查与勘探研究

中图分类号: P588.1;P597
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出版历程
- 收稿日期: 2017-08-22
- 刊出日期: 2018-07-15

Geochronology and Geochemistry of Volcanic Rocks from the Huangchengshan Volcanogenic Epithermal Silver Deposit, Dabie Orogen, China: Implications for Tectonic Setting

1.
Wuhan Center of China Geological Survey, Wuhan 430205, China
2.
Research Center of Granitic Diagenesis and Mineralization, China Geological Survey, Wuhan 430205, China
3.
Sixth Geological Brigade, Hubei Geological Bureau, Xiaogan 432000, China

摘要

摘要: 皇城山银矿床是西大别山地区代表性的浅成低温热液矿床，受陈棚组火山机构的枝叉状裂隙构造控制.目前人们对该矿床成因、成矿时间和构造环境的理解尚不深刻，因此对相关火山岩进行了激光等离子质谱（LA-ICP-MS）锆石U-Pb测年、元素地球化学和Sr-Nd-Hf同位素研究，探讨了其岩石成因和构造属性.结果表明，皇城山矿区陈棚组熔结凝灰岩及外围流纹岩锆石U-Pb年龄分别为133.4±1.5 Ma（MSWD=1.3）和133.1±0.8 Ma（MSWD=0.59），形成于早白垩世.陈棚组火山岩在较短时间内喷发形成，其喷发时限基本代表了皇城山银矿床形成时间.陈棚组流纹岩具高硅（SiO₂=73.83%~77.38%）、高钾（K₂O=4.65%~9.31%）特征，属于过铝质（A/CNK=1.09~1.31）和高钾钙碱性岩石系列.岩石具轻稀土富集，重稀土平坦，大离子亲石元素相对富集，Ba、Nb、Ta、P、Ti明显负异常和负Eu异常（δEu=0.33~0.88）特点.岩石锶同位素初始比值I_Sr为0.708 220~0.708 741，ε_Nd（t）值为-17.2~-18.5，Nd两阶段模式年龄T_DM2=2.32~2.43 Ga.锆石ε_Hf（t）值范围为-22.3~-26.1，Hf两阶段模式年龄T_DM2=2.29~2.49 Ga.主、微量元素和Sr-Nd-Hf同位素特征共同揭示陈棚组流纹岩为扬子陆壳北缘古老地壳物质重熔演化的产物.结合区域地质特征，陈棚组火山岩及其相关皇城山银矿床形成于大别山早白垩世加厚下地壳拆沉作用初期、挤压向伸展转化环境.
- 银矿床 /
- 火山岩 /
- 年代学 /
- 地球化学 /
- Sr-Nd-Hf同位素 /
- 大别山
Abstract: The Huangchengshan deposit is the largest high-sulfidation epithermal silver deposit in the Western Dabie orogen. Silver mineralization characterized by argentiferous quartz veins is controlled by fractures of volcanic apparatus, and is spatially associated with volcanic rocks of Chenpeng Formation. In situ zircon U-Pb dating yielded 133.4±1.5 Ma (1σ, MSWD=1.3) and 133.1±0.8 Ma (1σ, MSWD=0.59) for the tuff and rhyolite from Chenpeng Formation, respectively, indicating an Early Cretaceous volcanism. The data also suggest a syngenetic volcanogenic epithermal mineralization age of ca.133 Ma for the Huangchengshan silver deposit. Rhyolites of the Chenpeng Formation display high contents of SiO₂ (73.83% to 77.38%) and K₂O (4.65% to 9.31%), belonging to high-K calc-alkaline series. Their A/CNK ratios range from 1.09 to 1.31, exhibiting peraluminous characteristics. Rare earth elements show light rare earth elements (LREEs) enrichment and flat heavy rare earth elements (HREEs) patterns, with moderate negative Eu anomalies (δEu=0.33-0.88). They are enriched in large ion lithophile elements (LILEs), but depleted in Ba, Nb, Ta, P and Ti. These geochemical characteristics show affinity to highly fractionated granites. The rhyolites have high I_Sr values (0.708 220 to 0.708 741) and negative ε_Nd(t) values (-17.2 to -18.5), with two-stage Nd model ages of 2.32 to 2.43 Ga. Zircon ε_Hf(t) values are negative (-22.3 to -26.1) with an calculated two-stage Hf model ages of 2.29 to 2.49 Ga. The geochemical and Sr-Nd-Hf isotopic signatures suggest that the rhyolite is likely to be derived by partial melting of the ancient lower crust of the Yangtze Block. We propose that this volcanism and related Huangchengshan silver deposit formed in a transitional stage from crustal compression to extension driven by delamination of thickened lower crust during the Early Cretaceous.
- silver deposits /
- volcanic rocks /
- geochronology /
- geochemistry /
- Sr-Nd-Hf isotopes /
- Dabie orogen

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图 1 大别造山带北淮阳构造带火山岩分布及构造格架

据李双应(2004)；李鑫浩等(2015)修改

Fig. 1. Tectonic sketch of the northern Huaiyang belt showing the distribution of volcanic rocks

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图 2 皇城山银矿区地质简图

Fig. 2. Geological sketch of the Huangchengshan silver deposit

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图 3 陈棚组岩屑晶屑熔结凝灰岩(a, b)和流纹岩(c, d)野外和显微照片

a.赋矿陈棚组岩屑晶屑熔结凝灰岩野外照片，可见火山熔岩角砾和火山沉积构造；b.流纹岩野外照片；c.岩屑晶屑熔结凝灰岩单偏光显微照片，见火山沉积结构和气孔构造；d.流纹岩正交偏光显微照片，见斑状结构和气孔构造.Or.正长石；Pl.斜长石；Qz.石英

Fig. 3. Hand specimens and Photomicrographs of the ignimbrite (a, b) and rhyolite (c, d) from the Chenpeng Formation

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图 4 陈棚组熔结凝灰岩(a)和流纹岩(b)代表性锆石阴极发光(CL)图像

实线圆为锆石U-Pb测点，虚线圆为锆石Lu-Hf测点.图中锆石上方为测得U-Pb年龄，锆石下方为测得ε_Hf(t)值

Fig. 4. Cathodoluminescence (CL) images of representative zircons for the ignimbrite (a) and rhyolite (b) from the Chenpeng Formation

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图 5 陈棚组岩屑晶屑熔结凝灰岩(a, b)和流纹岩(c, d)锆石U-Pb年龄

岩屑晶屑熔结凝灰岩(样品HCS-1)的4颗捕获或继承锆石数据点未显示

Fig. 5. U-Pb concordia diagrams and weighted mean ages for the the ignimbrite (a, b) and rhyolite (c, d) from the Chenpeng Formation

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图 6 陈棚组流纹岩主量元素图解

陈棚组数据依据张四清等，1:5万文殊寺幅地质图说明书.河南省地质矿产勘查开发局第3地质调查队，2001年5月

Fig. 6. Major element diagrams for the rhyolite from the Chenpeng Formation

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图 7 陈棚组流纹岩稀土元素配分图(a)和微量元素原始地幔标准化蛛网图(b)

图a标准化值据Boynton(1984)；图b标准化值据Sun and Mcdonough(1989)

Fig. 7. Chondrite-normalized REE pattern (a) and primitive mantle-normalized trace elements diagram (b) for the rhyolite from the Chenpeng Formation

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图 8 陈棚组流纹岩和英安岩全岩Sr-Nd同位素组成

底图据John et al.(1999)、赵子福和郑永飞(2009)、陈伟等(2013)修改.数据来源：华北地块下地壳、中上地壳和扬子地块下地壳范围引自John et al.(1999)；中生代花岗岩范围赵子福和郑永飞(2009).陈棚组流纹岩数据为本文实测，英安岩数据杨梅珍等(2012)

Fig. 8. ε_Nd(t) vs. (⁸⁷Sr/⁸⁶Sr)_i diagram for the rhyolite from the Chenpeng Formation

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图 9 陈棚组流纹岩的锆石ε_Hf(t)-t图解

毛坦厂组安山岩锆石ε_Hf(t)数据为笔者实测(未发表)

Fig. 9. Zircon ε_Hf(t)-t vs. age diagram for the rhyolite from the Chenpeng Formation

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图 10 北淮阳晚中生代火山岩带不同地区火山岩形成时代

年龄数据同表 5

Fig. 10. Ages of the volcanic rocks in different tectonic units of the northern Huaiyang area, Dabie orogenic belt

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表 1 陈棚组火山岩LA-ICP-MS锆石U-Pb同位素测定结果

Table 1. LA-ICP-MS zircon isotopic U-Pb data for the volcanic rocks from the Chenpeng Formation

样品	元素含量(10^-6)				同位素比值						年龄(Ma)
样品	Pb	Th	U	Th/U	²⁰⁷Pb/²⁰⁶Pb	1σ	²⁰⁷Pb/²³⁵U	1σ	²⁰⁶Pb/²³⁸U	1σ	²⁰⁷Pb/²⁰⁶Pb	1σ	²⁰⁷Pb/²³⁵U	1σ	²⁰⁶Pb/²³⁸U	1σ
HCS-20：赋矿岩屑晶屑熔结凝灰岩
HCS-20@01	43	527	550	0.96	0.052 8	0.004 4	0.149 1	0.014 0	0.020 0	0.000 5	318	208	141	12	128	3
HCS-20@02	130	1 240	2 478	0.50	0.048 6	0.002 4	0.144 2	0.007 1	0.021 6	0.000 4	127	105	137	6	138	2
HCS-20@03	53	373	1 834	0.20	0.052 2	0.003 4	0.150 5	0.009 1	0.021 1	0.000 4	292	137	142	8	135	2
HCS-20@04	197	2 082	2 847	0.73	0.052 6	0.002 2	0.155 4	0.006 5	0.021 2	0.000 3	310	92	147	6	135	2
HCS-20@05	195	1 876	3 358	0.56	0.052 4	0.002 1	0.152 8	0.006 2	0.020 9	0.000 3	303	90	144	5	133	2
HCS-20@06	171	1 716	3 413	0.50	0.047 3	0.002 0	0.136 0	0.005 9	0.020 9	0.000 4	66	88	129	5	133	2
HCS-20@07	159	1 841	1 718	1.07	0.053 2	0.002 7	0.151 7	0.007 7	0.020 7	0.000 3	338	112	143	7	132	2
HCS-20@08	195	1 821	2 937	0.62	0.050 5	0.003 7	0.145 2	0.010 3	0.020 9	0.000 3	217	166	138	9	133	2
HCS-20@09	339	2 881	4 320	0.67	0.052 4	0.003 7	0.152 4	0.010 4	0.021 1	0.000 3	304	161	144	9	134	2
HCS-20@10	22	65	1 072	0.06	0.053 8	0.004 2	0.155 3	0.011 4	0.021 2	0.000 4	361	165	147	10	135	2
HCS-20@11	221	1 228	3 188	0.39	0.047 7	0.004 0	0.134 5	0.011 0	0.020 5	0.000 3	83	186	128	10	131	2
HCS-20@12	269	1 439	4 267	0.34	0.061 3	0.008 0	0.173 2	0.022 5	0.020 5	0.000 3	649	294	162	20	131	2
HCS-20@13	768	541	1 193	0.45	0.127 0	0.003 0	5.009 4	0.167 6	0.286 0	0.007 8	2 057	42	1 821	28	1 621	39
HCS-20@14	43	96	129	0.75	0.067 9	0.004 5	0.991 8	0.069 7	0.105 4	0.002 8	866	137	700	36	646	17
HCS-20@15	686	2 113	2 191	0.96	0.072 1	0.002 4	0.601 6	0.029 5	0.058 9	0.001 9	991	67	478	19	369	11
HCS-20@16	56	437	1 372	0.32	0.049 9	0.003 4	0.177 2	0.013 1	0.025 5	0.000 6	191	153	166	11	163	4
D001-3：流纹岩
D001-3@01	110	924	751	1.23	0.049 5	0.001 8	0.143 9	0.005 1	0.021 0	0.000 2	169	83	136	5	134	2
D001-3@02	423	3 691	1 849	2.00	0.049 3	0.001 4	0.140 9	0.003 9	0.020 7	0.000 2	161	64	134	3	132	1
D001-3@03	118	917	663	1.38	0.049 2	0.001 8	0.141 3	0.005 1	0.020 9	0.000 3	167	82	134	5	133	2
D001-3@04	362	3 159	1 685	1.88	0.049 4	0.001 3	0.142 2	0.004 0	0.020 8	0.000 2	165	63	135	4	132	1
D001-3@05	45	378	232	1.63	0.047 3	0.003 3	0.133 7	0.008 6	0.020 5	0.000 4	65	156	127	8	131	3
D001-3@06	233	1 937	1 309	1.48	0.049 1	0.001 5	0.139 4	0.004 5	0.020 5	0.000 2	154	77	132	4	131	2
D001-3@07	224	1 871	1 191	1.57	0.047 3	0.001 8	0.134 5	0.005 0	0.020 6	0.000 3	61	89	128	4	132	2
D001-3@08	280	2 375	1 471	1.61	0.049 3	0.001 4	0.142 3	0.004 1	0.020 9	0.000 2	161	64	135	4	133	1
D001-3@09	51	417	386	1.08	0.047 2	0.002 2	0.135 0	0.005 7	0.020 9	0.000 3	58	107	129	5	134	2
D001-3@10	242	1 884	1 231	1.53	0.049 9	0.001 4	0.144 1	0.004 2	0.020 9	0.000 3	191	65	137	4	133	2
D001-3@11	286	2 526	1 574	1.60	0.049 6	0.001 5	0.143 1	0.004 3	0.020 9	0.000 2	176	77	136	4	133	1
D001-3@12	160	1 332	927	1.44	0.048 7	0.002 1	0.140 3	0.006 0	0.020 9	0.000 3	132	99	133	5	133	2
D001-3@13	225	1 949	1 224	1.59	0.047 7	0.001 3	0.138 1	0.003 8	0.021 0	0.000 2	83	65	131	3	134	1
D001-3@14	52	440	283	1.56	0.049 6	0.003 6	0.140 6	0.009 5	0.020 9	0.000 4	176	168	134	8	133	2
D001-3@15	520	4 123	1 999	2.06	0.053 0	0.003 6	0.154 2	0.010 3	0.021 1	0.000 2	330	157	146	9	135	1

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表 2 陈棚组流纹岩主量元素(%)和微量、稀土元素(10^-6)分析结果

Table 2. Major elements (%), trace elements (10^-6) and rare earth elements (10^-6) of the rhyolite from the Chenpeng Formation

样号	D001-1	D001-2	D001-3	D001-4	D004-2
岩性	流纹岩	流纹岩	流纹岩	流纹岩	流纹岩
SiO₂	76.67	76.16	77.38	77.17	73.83
TiO₂	0.11	0.14	0.12	0.12	0.06
Al₂O₃	12.44	12.83	12.32	12.34	13.86
Fe₂O₃	0.72	0.78	0.63	0.55	0.91
FeO	0.63	0.58	0.52	0.55	0.58
MnO	0.05	0.04	0.04	0.03	0.03
MgO	0.15	0.16	0.12	0.12	0.22
CaO	0.36	0.30	0.28	0.28	0.10
Na₂O	3.04	3.50	3.38	3.34	0.22
K₂O	5.05	5.10	4.65	4.77	9.31
P₂O₅	0.02	0.02	0.02	0.03	0.03
Total	99.25	99.61	99.46	99.29	99.13
LOI	0.48	0.11	0.24	0.41	0.55
A/NK	1.19	1.14	1.16	1.16	1.33
A/CNK	1.12	1.09	1.11	1.11	1.31
La	27.80	34.50	20.10	20.30	4.08
Ce	45.50	56.30	37.10	35.80	8.27
Pr	4.02	5.37	3.00	3.01	1.07
Nd	9.34	13.50	7.05	7.12	3.16
Sm	1.38	2.13	1.05	1.05	0.63
Eu	0.14	0.23	0.13	0.13	0.15
Gd	1.22	1.69	0.94	0.94	0.43
Tb	0.18	0.26	0.15	0.15	0.08
Dy	1.10	1.55	0.93	0.96	0.44
Ho	0.24	0.31	0.21	0.22	0.09
Er	0.78	0.98	0.67	0.72	0.30
Tm	0.15	0.17	0.13	0.13	0.06
Yb	1.12	1.24	0.98	1.02	0.54
Lu	0.17	0.17	0.14	0.15	0.09
Y	7.48	8.99	6.35	6.59	3.59
Li	4.00	2.94	2.96	9.86	15.60
Cr	13.20	4.89	4.58	15.30	4.36
Co	1.54	2.05	1.08	<1	1.20
Ni	4.46	4.85	2.98	3.13	4.53
Ga	15.20	15.90	15.10	16.00	36.60
Nb	15.40	15.50	14.20	15.30	12.80
Mo	1.20	0.77	0.39	0.48	0.44
Ta	1.34	1.44	1.26	1.33	1.18
Th	8.66	11.00	8.67	22.00	32.30
U	3.46	4.96	2.63	3.11	14.90
Cl	53.80	58.70	80.40	45.60	82.00
Ba	75.20	157.00	189.00	186.00	354.00
Hf	4.46	4.67	4.23	4.47	16.50
Pb	36.70	42.60	92.10	113.00	69.00
Rb	176.00	156.00	141.00	159.00	570.00
Sr	42.60	113.00	53.30	52.20	22.60
Zr	85.40	99.60	80.30	86.60	152.00
Cs	1.74	1.45	1.04	1.09	11.50
As	1.01	0.78	0.70	0.78	3.66
Sb	0.17	0.10	0.16	0.10	0.32
Bi	0.07	0.05	0.23	0.20	0.25
Be	3.37	1.48	1.86	2.06	2.68
V	2.51	4.51	4.18	3.66	6.41
Sc	3.66	4.61	4.53	4.17	4.92
Cu	8.46	8.29	9.48	5.79	10.20
Zn	11.20	11.00	113.00	99.60	54.30
Au	0.46	0.59	0.51	0.56	11.90
Ag	0.09	0.07	0.24	0.13	56.00
F	337.00	439.00	210.00	634.00	892.00
∑REE	93.14	118.40	72.58	71.70	19.39
(La/Yb)_N	17.80	19.96	14.71	14.28	5.42
δEu	0.33	0.37	0.40	0.40	0.88
δCe	1.06	1.01	1.17	1.12	0.97

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表 3 陈棚组流纹岩全岩Sr-Nd同位素分析结果

Table 3. Whole rock Sr-Nd isotopic data of the rhyolite from the Chenpeng Formation

样品	岩石类型	年龄 (Ma)	Rb (10^-6)	Sr (10^-6)	⁸⁷Rb/ ⁸⁶Sr	⁸⁷Sr/ ⁸⁶Sr	I_Sr	Sm (10^-6)	Nd (10^-6)	¹⁴⁷Sm/ ¹⁴⁴Nd	¹⁴³Nd/ ¹⁴⁴Nd	(¹⁴³Nd/ ¹⁴⁴Nd)_i	ε_Nd(t)	T_DM2 (Ga)
D001-1	流纹岩	133	184.4	45.3	0.730 47	11.770	0.708 220	1.218	9.348	0.078 8	0.511 586	0.511 517	-18.5	2.43
D001-3	流纹岩	133	158.4	57.2	0.723 58	7.995	0.708 466	1.244	10.010	0.075 2	0.511 614	0.511 549	-17.9	2.38
D001-4	流纹岩	133	161.2	57.6	0.724 01	8.077	0.708 741	0.914	6.905	0.080 3	0.511 656	0.511 586	-17.2	2.32
注：计算过程所用参数(¹⁴⁷Sm/¹⁴³Nd)_CHUR=0.196 7；(¹⁴³Nd/¹⁴⁴Nd)_CHUR=0.512 638；(¹⁴⁷Sm/¹⁴³Nd)_DM=0.213 7；(¹⁴³Nd/¹⁴⁴Nd)_DM=0.513 15.

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表 4 陈棚组流纹岩的锆石Lu-Hf同位素LA-MC-ICP-MS原位分析结果

Table 4. LA-MC-ICP-MS zircon Lu-Hf isotopic data for the rhyolite from the Chenpeng Formation

样品点	年龄(Ma)	¹⁷⁶Lu/¹⁷⁷Hf	¹⁷⁶Yb/¹⁷⁷Hf	¹⁷⁶Hf/¹⁷⁷Hf	1σ	ε_Hf(0)	1σ	ε_Hf(t)	1σ	T_DM2(Ga)	f_Lu/Hf
D001-3@01	134	0.001 890	0.092 306	0.282 055	0.000 011	-25.4	0.7	-22.6	0.7	2.30	-0.94
D001-3@02	132	0.002 035	0.094 551	0.282 030	0.000 018	-26.2	0.8	-23.5	0.8	2.35	-0.94
D001-3@04	132	0.002 192	0.103 828	0.282 049	0.000 019	-25.6	0.8	-22.9	0.8	2.31	-0.93
D001-3@05	131	0.001 748	0.080 929	0.282 063	0.000 012	-25.1	0.7	-22.4	0.7	2.29	-0.95
D001-3@08	133	0.002 032	0.103 773	0.282 043	0.000 013	-25.8	0.7	-23.0	0.7	2.32	-0.94
D001-3@09	134	0.001 034	0.054 393	0.282 060	0.000 013	-25.2	0.7	-22.3	0.7	2.29	-0.97
D001-3@10	133	0.002 037	0.101 663	0.282 046	0.000 016	-25.7	0.8	-23.0	0.8	2.32	-0.94
D001-3@12	133	0.003 170	0.118 901	0.282 018	0.000 025	-26.7	1.0	-24.0	1.0	2.38	-0.90
D001-3@13	134	0.002 736	0.113 463	0.281 957	0.000 025	-28.8	1.0	-26.1	1.0	2.49	-0.92
D001-3@14	133	0.002 100	0.105 706	0.281 982	0.000 015	-27.9	0.7	-25.2	0.8	2.44	-0.94
注：测试点序号与表 1测年点序号对应.

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表 5 大别造山带北淮阳地区白垩纪火山岩年龄

Table 5. Ages of the Cretaceous volcanic rocks in the northern Huaiyang belt, Dabie orogenic belt

组名	岩性	年龄值(Ma)	测试方法	数据来源
陈棚组	石英安山岩	133.4±1.5	LA-ICP-MS锆石U-Pb	杨梅珍等(2012)
	熔结凝灰岩	133.1±1.5	LA-ICP-MS锆石U-Pb	本文
	流纹岩	133.1±0.8	LA-ICP-MS锆石U-Pb	本文
	英安斑岩	133.2±1.7	LA-ICP-MS锆石U-Pb	笔者实测，未发表
金刚台	粗安岩	129±2.0	SHRIMP锆石U-Pb	黄丹峰等(2010)
	正长斑岩	129.2±0.7	LA-ICP-MS锆石U-Pb	黄皓和薛怀民(2012)
	熔结凝灰岩	128.8±0.7	LA-ICP-MS锆石U-Pb	黄皓和薛怀民(2012)
	粗面安山岩	127.6±0.5	LA-ICP-MS锆石U-Pb	黄皓和薛怀民(2012)
	流纹岩	127±3.6	SHRIMP锆石U-Pb	黄丹峰等(2010)
	流纹英安岩	127.5±0.6	LA-ICP-MS锆石U-Pb	李鑫浩等(2015)
	英安岩	124.8±2.3	LA-ICP-MS锆石U-Pb	李鑫浩等(2015)
	安山岩	123.3±0.7	LA-ICP-MS锆石U-Pb	李鑫浩等(2015)
毛坦厂组	粗面质熔结凝灰岩	130.8±1.8	LA-ICP-MS锆石U-Pb	张定源等(2014)
毛坦厂组	安山岩	126.7±1.4	LA-ICP-MS锆石U-Pb	朱江等(2017)
晓天组	粗面岩	126.9±1.7	LA-ICP-MS锆石U-Pb	张定源等(2014)
望母山组	粗面岩	126.7±1.4	LA-ICP-MS锆石U-Pb	张定源等(2014)

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